Search results for "624 Civil engineering"
showing 4 items of 4 documents
Design, characterization, and first field deployment of a novel aircraft-based aerosol mass spectrometer combining the laser ablation and flash vapor…
2021
In this paper, we present the design, development, and characteristics of the novel aerosol mass spectrometer ERICA (ERC Instrument for Chemical composition of Aerosols; ERC – European Research Council) and selected results from the first airborne field deployment. The instrument combines two well-established methods of real-time in situ measurements of fine particle chemical composition. The first method is the laser desorption and ionization technique, or laser ablation technique, for single-particle mass spectrometry (here with a frequency-quadrupled Nd:YAG laser at λ = 266 nm). The second method is a combination of thermal particle desorption, also called flash vaporization, and electro…
Enhanced sulfur in the upper troposphere and lower stratosphere in spring 2020
2022
Sulfur compounds in the upper troposphere and lower stratosphere (UTLS) impact the atmosphere radiation budget, either directly as particles or indirectly as precursor gas for new particle formation. In situ measurements in the UTLS are rare but are important to better understand the impact of the sulfur budget on climate. The BLUESKY mission in May and June 2020 explored an unprecedented situation. (1) The UTLS experienced extraordinary dry conditions in spring 2020 over Europe, in comparison to previous years, and (2) the first lockdown of the COVID-19 pandemic caused major emission reductions from industry, ground, and airborne transportation. With the two research aircraft HALO and Falc…
Contribution of Asian emissions to upper tropospheric CO over the remote Pacific
2021
Abstract. Upon analysing the global distribution of the highest 2 % of daily CO mixing ratios at 400 hPa derived from the MOPITT satellite instrument for 20 years (2000–2019), we very regularly detect regions with very high CO values (i.e. mixing ratios belonging to the globally highest 2 %) over the remote Northern Hemispheric (NH) Pacific. Such events of elevated CO over the upper tropospheric NH Pacific occur throughout the year with surprisingly high regularity and frequency (70 % of all days during winter, 80 % of all days during spring). During winter, most of these pollution events are detected over the north-eastern and central NH Pacific, during spring over the central NH Pacific, …
Chemical analysis of the Asian tropopause aerosol layer (ATAL) with emphasis on secondary aerosol particles using aircraft-based in situ aerosol mass…
2022
Abstract. Aircraft-borne in situ measurements of the chemical aerosol composition were conducted in the Asian tropopause aerosol layer (ATAL) over the Indian subcontinent in the summer of 2017, covering particle sizes below ∼3 µm. We have implemented a recently developed aerosol mass spectrometer, which adopts the laser desorption technique as well as the thermal desorption method for quantitative bulk information (i.e., a modified Aerodyne AMS), aboard the high-altitude research aircraft M-55 Geophysica. The instrument was deployed in July and August 2017 during the StratoClim EU campaign (Stratospheric and upper tropospheric processes for better Climate predictions) over Nepal, India, Ban…